WANG Chen, SHEN Yan, ZHAO Xinghong, CHANG Zhiyuan, GUO Shilun, LIU Guorong, ZHAO Yonggang. Identification and Distinguishing of HEU Particle and Pu Particle by α Track Method[J]. Atomic Energy Science and Technology, 2020, 54(2): 366-372. DOI: 10.7538/yzk.2019.youxian.0139
Citation: WANG Chen, SHEN Yan, ZHAO Xinghong, CHANG Zhiyuan, GUO Shilun, LIU Guorong, ZHAO Yonggang. Identification and Distinguishing of HEU Particle and Pu Particle by α Track Method[J]. Atomic Energy Science and Technology, 2020, 54(2): 366-372. DOI: 10.7538/yzk.2019.youxian.0139

Identification and Distinguishing of HEU Particle and Pu Particle by α Track Method

More Information
  • The analytical technique of swipe sample particle analysis plays an important role in sample analysis of nuclear safeguard environmental sampling, and the first step of particle analysis is to search highly enriched uranium (HEU)bearing or Pu-bearing particles among dust particles. A new method for identifying HEU and Pu particles was established by using α track detection. First, an organic film containing particles was prepared and covered with a CR-39 solid state nuclear detector. After exposure, the detector was etched in a NaOH solution for different time, and the α track star parameters created by HEU or Pu particles were measured by optical microscope. The results show that the scatter plot of the dimeter of track end versus track minor axis can be used for HEU and Pu particles distinguishing when etching time is lager than 10 h, especially useful when track stars are concentrated.
  • [1]
    IAEA safeguards glossary, international nuclear verification series No.3[R]. Vienna: IAEA, 2001.
    [2]
    Environmental sampling for safeguards STR-348(Revision 1)[R]. Vienna: IAEA, 2011.
    [3]
    杨大助,傅秉一. 核不扩散与国际核保障核查[M].北京:中国原子能出版社,2012.
    [4]
    LEE M H, PARK J H, SONG K. Investigation on the nuclear track techniques for the screening of the fissile nuclides in swipe samples[J]. Radiation Measurements, 2011, 46: 409-412.
    [5]
    SHINNONAGA T, DONOHUE D, CIURAPINSKI A, et al. Age determination of single plutonium particles after chemical separation[J]. Spectrochimica Acta Part B, 2009, 64: 95-98.
    [6]
    HEDBERG P M L, PERES P, CLIFF J B, et al. Improved particle location and isotopic screening measurements of sub-micron sized particles by secondary ion mass spectrometry[J]. Journal of Analytical Atomic Spectrometry, 2011, 26: 406-413.
    [7]
    KUCHKIN A, LOMAKIN M, STEBELKOV V. Development of techniques for detection and subsequent analysis of alpha-emitting microparticles on fabrice, IAEA-TECDOC-1820[R]. Vienna: IAEA, 2017.
    [8]
    NOTO T, TOMITA H, KAWARABAYASHI J, et al. Preselecting method for plutonium particle analysis in environmental samples by nuclear emulsion[J]. Radiation Measurements, 2011, 46: 1807-1809.
    [9]
    邵自强. 硝化纤维素生产工艺及设备[M]. 北京:北京理工大学出版社,2002.
    [10]
    柳成林. 化学小组制赛璐珞软片的实验[J]. 化学通报,1958(1):60.
    [11]
    全国塑料标准化技术委员会. GB/T1033.1—2008塑料非泡沫塑料密度的测定,第1部分:浸渍法、液体比重瓶法和滴定法[S]. 北京:中国标准出版社,2009.

Catalog

    Article views (152) PDF downloads (1173) Cited by()

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return