Abstract: To deepen the knowledge of neutron albedo effect and get macroscopic measure data, the theoretical research of neutron albedo effect experiment was performed. The theoretical design of neutron albedo effect experiment was developed and the theoretical formula was determined. With two different experiment states, reaction rates of two nuclides under source neutron spectra and albedo neutron spectra can be measured. Then albedo effects by reaction rate of some measure points are quantified. The theoretical formula and the experiment layout scheme are effective. With experiment measure data, more quantitative informations of neutron albedo effect can be obtained.