Abstract:
For the preparation of ThO
2 pellet meeting to heavy water reactor (HWR) fuel element technical requirements, ThO
2 powder made by oxalic acid precipitation process was used as raw material. The ThO
2 pellet was prepared through the granulating, pressing and sintering process. The effects of granulating, pressing and sintering process on the grain size and density were analyzed. The results indicate that the specific surface area of powder, press force and sintering temperature are the main effect factors of pellet density. The driving forces of ThO
2 pellet sintering and grain growth increase with specific surface area of ThO
2 powder, and the ThO
2 pellet with larger grain size can be acquired by using the higher specific surface area of ThO
2 powder. The ThO
2 pellet which can meet the HWR fuel element technical requirements of density and grain size can be prepared under the vacuum or argon atmosphere and high sintering temperature.