提高HPGe γ能谱法测量131Xem133Xem探测灵敏度的方法研究

Method to Enhance Detection Sensitivities of 131Xem and 133Xem Measured by HPGe γ Spectrometer

  • 摘要: 放射性氙同位素(131Xem133Xem133Xe和135Xe)具有化学惰性、裂变产额大、易释放的特点,是监测核试验尤其是地下核试验最关键的核素之一。131Xem133Xem的γ射线发射概率小,X射线能量完全相同,致使HPGe γ能谱法测量131Xem133Xem活度的探测灵敏度低。针对这一技术难题,本文研究建立了131Xem133Xem活度测量的X/γ射线交互分析方法。利用贝叶斯方法推导了γ能谱中净峰面积概率分布,根据得到的131Xem133XemX射线和γ射线净峰面积分布构建了活度分布的似然函数,采用最大似然法得到了131Xem133Xem活度。相对于仅用γ射线分析,提高了131Xem133Xem的探测灵敏度。

     

    Abstract: Owing to their inert chemical properties, large fission yields, and abilities to easily vent into the atmosphere, detection of radioactive xenon isotopes (131Xem, 133Xem, 133Xe and 135Xe) is one of the most effective technology of underground test monitoring. Due to the lower γ ray emission probability and energy overlapping of X ray, the detection sensitivities of 131Xem and 133Xem are lower measured by using HPGe γ spectrometer. To enhance the detection sensitivities of 131Xem and 133Xem, an X and γ ray interactive analysis method was developed. The distribution of the net peak counts in γ spectrum was deduced through Bayesian approach. The likelihood function of 131Xem and 133Xem activities was established by using the distribution of net peak counts of X and γ ray. The activities of 131Xem and 133Xem were estimated by maximum likelihood method. The detection sensitivities of 131Xem and 133Xem are enhanced comparing with analyzing their γ ray.

     

/

返回文章
返回