铀矿石浓缩物的地理溯源特征属性分析技术研究现状

Research Status of Geological Traceability Analysis of Uranium Ore Concentrate

  • 摘要: 近年来随着核法证分析技术的发展,基本确定了铀同位素、稀土元素(REE)分布模式、Sr和Nd同位素丰度、部分杂质元素含量等为铀矿石浓缩物(UOC)地理溯源特征指纹,高准确性、高精度的分析方法为溯源提供了技术支撑。主要的技术发展体现在,根据不同类型的UOC样品采用不同的溶解及化学分离方法,先进质谱技术发展在UOC中铀及杂质的含量及同位素等地理特征属性测量中的应用,及基体一致的UOC标准样品在溶解、分离、测量全过程中质量控制的保障。为推动核化学、地质化学等在核法证技术中的应用,本文基于近年来国内外的研究成果,对UOC的核法证地理溯源分析技术发展、数据处理进行了详细论述。

     

    Abstract: In recent years, with the development of nuclear forensic analysis technology supported by high-accuracy and high-precision analysis methods, uranium isotopes, the distribution pattern of rare earth elements (REE), Sr and Nd isotope abundances, and some impurity element contents are mainly identified as effective geographic traceability fingerprint information of uranium ore concentrate (UOC). The main technological developments include different dissolution and chemical separation methods depending on the types of UOC samples, the advanced mass spectrometry technology used in the measurement of geographic characteristics such as the content and isotopic abundance of uranium and impurities in UOC, and the UOC standard samples with the same matrix as quality control (QC) measure used in the entire process of dissolution, separation and measurement. To promote the application of nuclear chemistry and geochemistry etc. in the study of nuclear forensics, based on the research achievements in recent years, the details of development in UOC’s nuclear forensic geographic traceability analysis technology and data processing are discussed.

     

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