56Fe核数据对屏蔽计算不确定度的影响研究

Influence of Nuclear Data of 56Fe on Shielding Calculation Uncertainty

  • 摘要: 56Fe是反应堆屏蔽设计中的重要核素之一,量化56Fe对屏蔽计算造成的不确定度,对确定反应堆屏蔽设计不确定度来源具有重要意义。本文首先利用评价核数据库抽样程序NECP-SOUL,基于JEFF-3.3、ENDF/B-Ⅷ.0进行抽样,然后对每个样本利用核数据处理程序NECP-Atlas制作适用于屏蔽计算的多群数据库,利用离散纵标输运程序NECP-hydra计算ASPIS-Fe与ALARM-CF-FE-SHIELD-001基准题,量化探测器反应率计算结果的不确定度。结果表明,随屏蔽材料厚度的增加,不确定度逐渐增大;仅对截面协方差进行抽样时,弹性散射与非弹性散射截面协方差对快中子探测器反应率不确定度有较大影响,对1 MeV以上中子敏感的32S(n,p)32P探测器造成的不确定度最大达20%以上;此外,在同时考虑截面协方差与次级粒子角分布协方差后,不确定度量化结果会比仅考虑截面协方差时增加约2%。

     

    Abstract: 56Fe is one of important nuclides in reactor shielding design. Quantifying the uncertainty introduced by the nuclear data of 56Fe in shielding calculation is significant for determining the sources of uncertainty in reactor shielding design. The nuclear data library used for shielding calculation is generated based on the evaluated nuclear data file (ENDF). The generation of ENDF involves processes such as theoretical calculations, experimental measurements, and data evaluation testing. Inevitably, there is uncertainty in these processes, which leads to uncertainty in the calculation results. In this present work, the uncertainty of a couple of benchmarks caused by the nuclear data of 56Fe was analyzed. The uncertainty quantification process was composed of the three steps. First, the NECP-SOUL code was used to generate random samples of ENDF based on the best estimates and covariance from JEFF-3.3 and ENDF/B-Ⅷ.0 evaluated nuclear data files, respectively. After constructing the covariance matrix from the ENDF, an improved Latin hypercube sampling technique was used to generate normally distributed nuclear data samples. Second, the ENDF samples were processed using nuclear data processing code NECP-Atlas to generate the multi-group cross section library. For the energy group structure of the multi-group library, the VITAMIN-B6 energy group structure was selected. Due to the strong resonance of the cross section of 56Fe and other nuclides in structural materials, the resonance self-shielding effect makes the multi-group cross-sections dependent on the temperature, geometry, and material composition of the actual problem. Therefore, resonance self-shielding calculations were performed based on the actual problem to generate a problem-dependent multi-group cross section library. Third, the ASPIS-Fe benchmark and ALARM-CF-FE-SHIELD-001 benchmark were calculated using the discrete ordinate based neutron transport code NECP-hydra, and the uncertainty in the detector reaction rate calculation results was quantified based on the results obtained using all the library samples. The results show that the elastic and inelastic scattering cross section has significant impact on the uncertainty of fast neutron detector reaction rates. The uncertainty of the response of 32S(n,p)32P detector, which sensitive to neutron over 1 MeV, can reach over 20%. In addition, when both the covariance of cross section and the secondary angular distribution are considered, the uncertainty quantification results increase by approximately 2% compared to the case where only the cross section covariance is considered.

     

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